Grey (alternative spelling "gray"), in general, has negative connotations. There is grey: hair (a loss of youth and vitality), skies (gloomy), complexion (lack of health and vigor), environment (lack of color and vibrancy).
Grey eyes also connote "steely eyes," which, though determined, lack warmth and compassion.
If I wanted to compliment someone with grey eyes, I would tell them they have "beautiful pale blue eyes!"